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81.
Asymmetric-Flow Field-Flow Fractionation (AsFlFFF) coupled to an inductively coupled plasma-mass spectrometer (ICP-MS) was used to determine whether colloidal As exists in mine tailings from abandoned Au mine sites in Nova Scotia. Using this technique, the chemical composition and the size of the colloidal material was determined. Tailings samples were collected from the sites and leachates were analyzed. The resulting fractograms showed the presence of colloidal As. Arsenic co-elutes with Fe and Al suggesting that the As is associated with colloids containing these elements. The colloidal material present in the samples has a calculated median size of 7 nm. The leachates were also analyzed for totalAs, Fe and Al using ICP-MS. The colloidal fraction was determined to account for approximately 20% of the total dissolved As present in these samples. Dissolved As concentrations at the selected mine sites are very high and the arbitrary cutoff for dissolved still incorporates colloidal material. Therefore. it is important to distinguish between truly dissolved and colloidal As as the speciation will affect the toxicity and mobility of As at these locations. 相似文献
82.
Kord Ernstson Werner Mayer Andreas Neumair Dirk Sudhaus 《Central European Journal of Geosciences》2011,3(4):385-397
Sudden collapse of the Quaternary soil to form sinkholes on the order of meters and tens of meters has been a geologic phenomenon within living memory in a localized area north of Lake Chiemsee in Southeast Germany. Failing a satisfying explanation, a relation with an undefined glaciation process has always been proposed. Excavations and geophysical measurements at three newly affected sites show underground features such as prominent sandy-gravelly intrusions and extrusions typical of rock liquefaction processes well known to occur during strong earthquakes. Since strong earthquakes can reasonably be excluded to have affected the area under discussion, it has been suggested that the observed widespread liquefaction is related with the recently proposed Holocene Chiemgau meteorite impact event. Except for one earlier proposed but unassertive relation between impact and liquefaction, the obviously direct association of both processes in the Chiemgau area emphasizes that observed paleoliquefaction features need not necessarily have originated solely from paleoseismicity but can provide a recognizable regional impact signature. 相似文献
83.
Dirk Schories Karsten Reise Karen Sanamyan Nadya Sanamyan Elena Clasing Anneken Reise 《Journal of Sea Research》2011,65(2):304-314
Generally, estuarine intertidal mudflats constitute important nurseries for fish and foraging grounds for coastal birds by providing a plenitude of mollusks, worms, and crustaceans as prey, which in turn mostly feed on suspended and benthic microalgae, bacteria, and detritus. Despite the high productivity of such habitats, pronounced variability in both salinity and temperature results typically in low diversity. The only sea anemone reported from estuarine mud is the edwardsiid Nematostella vectensis Stephenson, 1935. It occurs widely in the northern hemisphere, and occasionally in extremely high density. Here we document another sea anemone from estuarine mud and muddy sand found in Southern Chile which has similar ecological attributes. Taxonomic confusion has impeded the reporting on this small but prominent member in a macrozoobenthic assemblage, the brooding Anthopleura hermaphroditica (Carlgren, 1899; Anthozoa: Actiniidae). It differs from N. vectensis by the presence of symbiotic algae. Average density under poly- to euhaline conditions in mud and muddy sand at around mid tide level was about 3 actinians per cm2. An average abundance of 11,000 m? 2, a biovolume of 487 cm3 m? 2, and a biomass of 35.5 g dry organic weight m? 2 were found in mud and muddy sand in two surveys 20 years apart. The mean fishing area of fully expanded individuals covers 42 ± 25 mm2, corresponding to a circular area with a diameter of 7.3 ± 5.7 mm. Preliminary experiments indicate that associated benthos may be relegated to life below surface by the net of tentacles above the sediment. As no predators on A. hermaphroditica could be found on the mudflat, the success of this mixotrophic sea anemone may entail a trophic dead end. 相似文献
84.
James U.L. Baldini Frank McDermott Dirk L. Hoffmann David A. Richards Nicholas Clipson 《Earth and Planetary Science Letters》2008,272(1-2):118-129
Cave air PCO2 at two Irish sites varied dramatically on daily to seasonal timescales, potentially affecting the timing of calcite deposition and consequently climate proxy records derived from stalagmites collected at the same sites. Temperature-dependent biochemical processes in the soil control CO2 production, resulting in high summer PCO2 values and low winter values at both sites. Large Large-amplitude, high-frequency variations superimposed on this seasonal cycle reflect cave air circulation. Here we model stalagmite growth rates, which are controlled partly by CO2 degassing rates from drip water, by considering both the seasonal and high-frequency cave air PCO2 variations. Modeled hourly growth rates for stalagmite CC-Bil from Crag Cave in SW Ireland reach maxima in late December (0.063 μm h− 1) and minima in late June/early July (0.033 μm h− 1). For well-mixed ‘diffuse flow’ cave drips such as those that feed CC-Bil, high summer cave air PCO2 depresses summer calcite deposition, while low winter PCO2 promotes degassing and enhances deposition rates. In stalagmites fed by well-mixed drips lacking seasonal variations in δ18O, integrated annual stalagmite calcite δ18O is unaffected; however, seasonality in cave air PCO2 may influence non-conservative geochemical climate proxies (e.g., δ13C, Sr/Ca). Stalagmites fed by ‘seasonal’ drips whose hydrochemical properties vary in response to seasonality may have higher growth rates in summer because soil air PCO2 may increase relative to cave air PCO2 due to higher soil temperatures. This in turn may bias stalagmite calcite δ18O records towards isotopically heavier summer drip water δ18O values, resulting in elevated calcite δ18O values compared to the ‘equilibrium’ values predicted by calcite–water isotope fractionation equations. Interpretations of stalagmite-based paleoclimate proxies should therefore consider the consequences of cave air PCO2 variability and the resulting intra-annual variability in calcite deposition rates. 相似文献
85.
86.
Stefan Jansen Eva Walpersdorf Ursula Werner Markus Billerbeck Michael E Böttcher Dirk de Beer 《Ocean Dynamics》2009,59(2):317-332
In this article, we describe the dynamics of pH, O2 and H2S in the top 5–10 cm of an intertidal flat consisting of permeable sand. These dynamics were measured at the low water line
and higher up the flat and during several seasons. Together with pore water nutrient data, the dynamics confirm that two types
of transport act as driving forces for the cycling of elements (Billerbeck et al. 2006b): Fast surface dynamics of pore water chemistry occur only during inundation. Thus, they must be driven by hydraulics (tidal
and wave action) and are highly dependent on weather conditions. This was demonstrated clearly by quick variation in oxygen
penetration depth: Seeps are active at low tide only, indicating that the pore water flow in them is driven by a pressure
head developing at low tide. The seeps are fed by slow transport of pore water over long distances in the deeper sediment.
In the seeps, high concentrations of degradation products such as nutrients and sulphide were found, showing them to be the
outlets of deep-seated degradation processes. The degradation products appear toxic for bioturbating/bioirrigating organisms,
as a consequence of which, these were absent in the wider seep areas. These two mechanisms driving advection determine oxygen
dynamics in these flats, whereas bioirrigation plays a minor role. The deep circulation causes a characteristic distribution
of strongly reduced pore water near the low water line and rather more oxidised sediments in the centre of the flats. The
two combined transport phenomena determine the fluxes of solutes and gases from the sediment to the surface water and in this
way create specific niches for various types of microorganisms. 相似文献
87.
88.
Field experiments were conducted in Nellis Dunes Recreational Area (Clark County, Nevada, USA) to investigate emission of dust produced by off-road driving. Experiments were carried out with three types of vehicles: 4-wheelers (quads), dirt bikes (motorcycles) and dune buggies, on 17 soil types characteristic for a desert environment. Tests were done at various driving speeds, and emissions were measured for a large number of grain size fractions. This paper reports the results for two size fractions of emissions: PM10 (particles < 10 μm) and PM60 (particles < 60 μm). The latter was considered in this study to be sufficiently representative of the total suspendable fraction (TSP). Off-road driving was found to be a significant source of dust. However, the amounts varied greatly with the type of soil and the characteristics of the top layer. Models predicting emission of dust by off-road driving should thus consider a number of soil parameters and not just one key parameter. Vehicle type and driving speed are additional parameters that affect emission. In general, 4-wheelers produce more dust than dune buggies, and dune buggies, more than dirt bikes. Higher speeds also result in higher emissions. Dust emitted by off-road driving is less coarse than the parent sediment on the road surface. Off-road driving thus results in a progressive coarsening of the top layer. Exceptions to this are silty surfaces with no, or almost no, vegetation. For such surfaces no substantial differences were observed between the grain size distribution of road dust and emitted dust. Typical emission values for off-road driving on dry desert soils are: for sandy areas, 30–40 g km− 1 (PM10) and 150–250 g km− 1 (TSP); for silty areas, 100–200 g km− 1 (PM10) and 600–2000 g km− 1 (TSP); for drainages, 30–40 g km− 1 (PM10) and 100–400 g km− 1 (TSP); and for mixed terrain, 60–100 g km− 1 (PM10) and 300–800 g km− 1 (TSP). These values are for the types of vehicles tested in this study and do not refer to cars or trucks, which produce significantly more dust. 相似文献
89.
Dirk Kossow Charlotte Krawczyk Tommy McCann Manfred Strecker Jörg F.W. Negendank 《International Journal of Earth Sciences》2000,89(3):652-664
The northern part of the Northeast German Basin contains a large number of Late Permian (Zechstein) salt pillows, whereas diapiric structures are almost completely absent. This lack of diapirs facilitated the study of early stages of salt movement in the basin. Salt pillows and related structures were investigated in terms of distribution, geometry and time of initiation of salt flow within the regional geological context. The primary Zechstein thickness in the study area was reconstructed to gain more insight into the relationship between the geometry of the salt layer and the style of the salt-related structures. In this study, no clear spatial relationship between the salt structures and basement faults has been found and the location of the salt structures in this area appears to be highly independent of the underlying structural grain. The overburden is affected by minor faulting. We propose that buckling of the overburden due to regional compression significantly contributed to the initiation of the Late Jurassic to Early Cretaceous salt structures in the basin. Reverse faulting of the Gardelegen and Haldensleben Faults is related to inversion tectonics and exerted a compression on the basin fill. During the deformation, the Late Permian salt layer acted as an efficient detachment and led to a marked decoupling of the Mesozoic overburden from the underlying pre-Zechstein rocks. 相似文献
90.